- By:
- Klemm, Mason; Zhang, Tingjun; Winn, Barry L; Li, Fankang ; Ye, Feng ; Matsuda, Masaaki ; Maity, Avishek ; Xu, Sijie; Teng, Xiaokun; Umemoto, Yoshihiko ; Gao, Bin; Yi, Ming; Dai, Pengcheng
- Journal Name:
- Physical Review B
- Page Number:
- 174422
- Volume:
- 112
- Publication Date:
- November 26, 2025
- View DOI Listing:
- https://doi.org/10.1103/d88l-4wq8
Abstract
Unveiling the interplay between spin density wave (SDW) and charge density wave (CDW) orders in correlated electron materials is important in obtaining a comprehensive understanding of their electronic, structural, and magnetic properties. Kagome lattice materials are interesting because their flat electronic bands, Dirac points, and Van Hove singularities can enable a variety of exotic electronic and magnetic phenomena. The kagome metal FeGe (the B35 phase), which exhibits a CDW order deep within an A-type antiferromagnetic (AFM) phase, was found to respond dramatically to postgrowth annealing—with the ability to tune the CDW repeatedly from long-range order to negligible order. Additionally, neutron scattering studies suggest that incommensurate magnetic peaks that onset at 𝑇Canting=𝑇SDW≈60K in the system arise from a SDW order instead of the AFM double-cone structure. Here we use inelastic neutron scattering to show that two distinct spin excitations exist below 𝑇Canting corresponding to two coexisting magnetic orders in the system in both sets of annealed samples with and without CDW. While CDW order or negligible order can dramatically affect the onset temperature of 𝑇Canting and elastic incommensurate magnetic scattering, its impact on low-energy spin fluctuations is more limited. In both samples, a pair of gapless incommensurate spin excitations arising from the SDW order wave vector coexist with gapped commensurate spin waves from the A-type AFM order across 𝑇Canting. The low-energy spin excitations for both samples couple dynamically to the lattice through enhanced magnetic scattering intensity on cooling below 𝑇CDW, regardless of the status of the static long-range CDW order. The incommensurate SDW order in the long-range CDW ordered sample also induces a tiny in-plane lattice distortion of the kagome lattice that is absent in the negligible CDW ordered sample, in a way that is different from the previously known SDW and CDW ordering materials.
